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Charge exchange and spectroscopy with isolated
             highly-charged ions
                   Nicholas D. Guise
          Samuel M. Brewer, Joseph N. Tan
              Quantum Measurement Division
        National Institute of Standards and Technology
                   Gaithersburg, MD 20899




                         8 June 2012
Overview
  Goal
Engineer highly-charged ions (HCI) of interest in metrology, astrophysics,
plasma diagnostics, and collision studies


                                                q/m
  Basic Scheme                                  analyzing
                                                magnet
                                                                      fs comb
 1) Extract HCI from EBIT source                             ion
 2) Recapture in Penning trap                                trap     laser
                                               ions
 3) Study recaptured ions
    -charge exchange
    -optical spectroscopy
                                                   CX beam
                                                                    MCP detector



                                         EBIT
                               (electron beam ion trap)
Permanent Magnet Penning Traps




            One-Magnet Trap                                      Two-Magnet Trap
• B field provided by one NdFeB magnet              • B field more homogeneous near center
• Magnet also functions as ring electrode           • Holes in ring provide optical access
• Simple construction with copper endcaps           • Iron electrodes shape field profile

                           J.N. Tan, S.M. Brewer, and N.D. Guise, Rev. Sci. Instrum. 83, 023103 (2012)
Experiment Region
              TOF Detector:
              8 mm diameter
                                                            Photomultiplier
              <1 ns rise time
                                                            Tube

Ne10+ Beam Spot            Time-of-Flight
on Position-
Sensitive MCP              MCP Detector
                           (TOF), on
                           retractable translator




 XY Position
 Sensitive MCP                                                                           1-Magnet
 Detector                                                                                Penning Trap



                                                                          2-Magnet
                                                    RF Trap/              Penning Trap
                                                    Lens/Filter
Ion Capture and Detection
t=0                              t=tcapture ≈ 17 µs          t=tstorage ≈ 200ms       t ≈ tstorage+1 µs
extract ions                     pulse trap closed           pulse trap open          ions arrive at MCP
from EBIT                        to capture ions             to dump ions             detector




EBIT                                                                                            MCP
                                  capture




                                                                               dump
               applied voltage




                                  Front Endcap        Ring         Back Endcap
Ion Extraction and Capture Timing
Ion Energy




             Ion energy
             ~ 5.5 eV
Ion Charge Exchange

          sum of all         bare Ne        charge state evolution
          charge states      nuclei



                              H-like
                              Ne


                              He-like
 Ne10+                        Ne                     bare Ne
 only                                                nuclei




     Parameters                             H-like
  Two-Magnet Trap                           Ne                 He-like
                                                               Ne
    V0 ≈ 2.5 kV
∆V=Vring-Vendcap = 25 V
Ion Storage: Pressure Dependence
       Parameters
     Two-Magnet Trap
       V0≈ 2.5 kV
   ∆V=Vring-Vendcap = 25 V
Long-Term Focus: H-like ions in Circular
                   Rydberg States

                                       • Theory more accurate than for
     Electron Probability                Hydrogen S states due to:
         Distribution                     • negligible interactions with the nucleus
                                          • accuracy of calculated corrections, including
                                            QED effects
                                       • |n› → |n-1› transitions are accessible
                                         to optical frequency comb


nucleus: Ze+
           electron state: | n,l,m ›
              |m|=l=n-1




                                          U.D. Jentschura, P.J. Mohr, J.N. Tan, and B.J. Wundt,
                                          Phys. Rev. Lett. 100, 160404 (2008).
New Apparatus for Low Charge States




Electron
gun         Ion                                    18 mm
            production                             TOF detector
            region
                               Experiment region
                               with two-magnet
                               Penning trap
Summary

• Unitary architecture NdFeB Penning traps are used to capture and
  store highly charged ions extracted from the NIST EBIT.
• Captured ion species include Ne10+, Ne9+, Ne8+, Ar16+, Ar15+, Ar14+,
  Ar13+, N7+, and Kr17+.
• Ion storage times of order 1 second are limited primarily by collisions
  with residual gas at 300 K.
• Ongoing experiments include studies of charge exchange, optical
  measurements of metastable lifetimes (upcoming talk by S. Brewer).
• New apparatus will utilize similar NdFeB construction for a room-
  temperature “mini-EBIT” source, for planned spectroscopy with low-Z
  hydrogen-like ions.

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Charge exchange and spectroscopy with isolated highly-charged ions

  • 1. Charge exchange and spectroscopy with isolated highly-charged ions Nicholas D. Guise Samuel M. Brewer, Joseph N. Tan Quantum Measurement Division National Institute of Standards and Technology Gaithersburg, MD 20899 8 June 2012
  • 2. Overview Goal Engineer highly-charged ions (HCI) of interest in metrology, astrophysics, plasma diagnostics, and collision studies q/m Basic Scheme analyzing magnet fs comb 1) Extract HCI from EBIT source ion 2) Recapture in Penning trap trap laser ions 3) Study recaptured ions -charge exchange -optical spectroscopy CX beam MCP detector EBIT (electron beam ion trap)
  • 3. Permanent Magnet Penning Traps One-Magnet Trap Two-Magnet Trap • B field provided by one NdFeB magnet • B field more homogeneous near center • Magnet also functions as ring electrode • Holes in ring provide optical access • Simple construction with copper endcaps • Iron electrodes shape field profile J.N. Tan, S.M. Brewer, and N.D. Guise, Rev. Sci. Instrum. 83, 023103 (2012)
  • 4. Experiment Region TOF Detector: 8 mm diameter Photomultiplier <1 ns rise time Tube Ne10+ Beam Spot Time-of-Flight on Position- Sensitive MCP MCP Detector (TOF), on retractable translator XY Position Sensitive MCP 1-Magnet Detector Penning Trap 2-Magnet RF Trap/ Penning Trap Lens/Filter
  • 5. Ion Capture and Detection t=0 t=tcapture ≈ 17 µs t=tstorage ≈ 200ms t ≈ tstorage+1 µs extract ions pulse trap closed pulse trap open ions arrive at MCP from EBIT to capture ions to dump ions detector EBIT MCP capture dump applied voltage Front Endcap Ring Back Endcap
  • 6. Ion Extraction and Capture Timing
  • 7. Ion Energy Ion energy ~ 5.5 eV
  • 8. Ion Charge Exchange sum of all bare Ne charge state evolution charge states nuclei H-like Ne He-like Ne10+ Ne bare Ne only nuclei Parameters H-like Two-Magnet Trap Ne He-like Ne V0 ≈ 2.5 kV ∆V=Vring-Vendcap = 25 V
  • 9. Ion Storage: Pressure Dependence Parameters Two-Magnet Trap V0≈ 2.5 kV ∆V=Vring-Vendcap = 25 V
  • 10. Long-Term Focus: H-like ions in Circular Rydberg States • Theory more accurate than for Electron Probability Hydrogen S states due to: Distribution • negligible interactions with the nucleus • accuracy of calculated corrections, including QED effects • |n› → |n-1› transitions are accessible to optical frequency comb nucleus: Ze+ electron state: | n,l,m › |m|=l=n-1 U.D. Jentschura, P.J. Mohr, J.N. Tan, and B.J. Wundt, Phys. Rev. Lett. 100, 160404 (2008).
  • 11. New Apparatus for Low Charge States Electron gun Ion 18 mm production TOF detector region Experiment region with two-magnet Penning trap
  • 12. Summary • Unitary architecture NdFeB Penning traps are used to capture and store highly charged ions extracted from the NIST EBIT. • Captured ion species include Ne10+, Ne9+, Ne8+, Ar16+, Ar15+, Ar14+, Ar13+, N7+, and Kr17+. • Ion storage times of order 1 second are limited primarily by collisions with residual gas at 300 K. • Ongoing experiments include studies of charge exchange, optical measurements of metastable lifetimes (upcoming talk by S. Brewer). • New apparatus will utilize similar NdFeB construction for a room- temperature “mini-EBIT” source, for planned spectroscopy with low-Z hydrogen-like ions.